| #1 | 08/10/1961 | Luxembourg | - | Portugal | 4:2 |  |
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| #2 | 25/10/1961 | England | - | Portugal | 2:0 | ||||
| #3 | 06/05/1962 | Brazil | - | Portugal | 2:1 | ||||
| #4 | 09/05/1962 | Brazil | - | Portugal | 1:0 | ||||
| #5 | 17/05/1962 | Portugal | - | Belgium | 1:2 | |
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| #6 | 07/11/1962 | Bulgaria | - | Portugal | 3:1 | |
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| #7 | 16/12/1962 | Portugal | - | Bulgaria | 3:1 | ||||
| #8 | 21/04/1963 | Portugal | - | Brazil | 1:0 | ||||
| #9 | 29/04/1964 | Switzerland | - | Portugal | 2:3 | ||||
| #10 | 03/05/1964 | Belgium | - | Portugal | 1:2 | |
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| #11 | 17/05/1964 | Portugal | - | England | 3:4 | |
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| #12 | 31/05/1964 | Portugal | - | Argentina | 0:2 | ||||
| #13 | 04/06/1964 | Portugal | - | England | 1:1 | ||||
| #14 | 15/11/1964 | Portugal | - | Spain | 2:1 | |
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| #15 | 24/01/1965 | Portugal | - | Turkey | 5:1 | |
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| #16 | 19/04/1965 | Turkey | - | Portugal | 0:1 | |
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| #17 | 25/04/1965 | CSSR | - | Portugal | 0:1 | |
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| #18 | 13/06/1965 | Portugal | - | Romania | 2:1 | |
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| #19 | 24/06/1965 | Portugal | - | Brazil | 0:0 | ||||
| #20 | 31/10/1965 | Portugal | - | CSSR | 0:0 | ||||
| #21 | 21/11/1965 | Romania | - | Portugal | 2:0 | ||||
| #22 | 12/06/1966 | Portugal | - | Norway | 4:0 | |
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| #23 | 18/06/1966 | Scotland | - | Portugal | 0:1 | ||||
| #24 | 21/06/1966 | Denmark | - | Portugal | 1:3 | |
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| #25 | 26/06/1966 | Portugal | - | Uruguay | 3:0 | ||||
| #26 | 03/07/1966 | Portugal | - | Romania | 1:0 | ||||
| #27 | 13/07/1966 | Portugal | - | Hungary | 3:1 | ||||
| #28 | 16/07/1966 | Portugal | - | Bulgaria | 3:0 | |
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| #29 | 19/07/1966 | Portugal | - | Brazil | 3:1 | |
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| #30 | 23/07/1966 | Portugal | - | North Korea | 5:3 | |
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| #31 | 26/07/1966 | England | - | Portugal | 2:1 | |
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| #32 | 28/07/1966 | Portugal | - | USSR | 2:1 | |
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| #33 | 13/11/1966 | Portugal | - | Sweden | 1:2 | ||||
| #34 | 27/03/1967 | Italy | - | Portugal | 1:1 | |
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| #35 | 01/06/1967 | Sweden | - | Portugal | 1:1 | ||||
| #36 | 08/06/1967 | Norway | - | Portugal | 1:2 | |
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| #37 | 12/11/1967 | Portugal | - | Norway | 2:1 | ||||
| #38 | 26/11/1967 | Bulgaria | - | Portugal | 1:0 | ||||
| #39 | 17/12/1967 | Portugal | - | Bulgaria | 0:0 | ||||
| #40 | 27/10/1968 | Portugal | - | Romania | 3:0 | ||||
| #41 | 11/12/1968 | Greece | - | Portugal | 4:2 | |
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| #42 | 16/04/1969 | Portugal | - | Switzerland | 0:2 | ||||
| #43 | 04/05/1969 | Portugal | - | Greece | 2:2 | |
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| #44 | 12/10/1969 | Romania | - | Portugal | 1:0 | ||||
| #45 | 02/11/1969 | Switzerland | - | Portugal | 1:1 | |
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| #46 | 14/10/1970 | Denmark | - | Portugal | 0:1 | ||||
| #47 | 17/02/1971 | Belgium | - | Portugal | 3:0 | ||||
| #48 | 21/04/1971 | Portugal | - | Scotland | 2:0 | |
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| #49 | 12/05/1971 | Portugal | - | Denmark | 5:0 | |
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| #50 | 13/10/1971 | Scotland | - | Portugal | 2:1 | ||||
| #51 | 21/11/1971 | Portugal | - | Belgium | 1:1 | ||||
| #52 | 29/03/1972 | Portugal | - | Cyprus | 4:0 | ||||
| #53 | 11/06/1972 | Portugal | - | Ecuador | 3:0 | |
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| #54 | 14/06/1972 | Portugal | - | Iran | 3:0 | |
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| #55 | 18/06/1972 | Portugal | - | Chile | 4:1 | |
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| #56 | 25/06/1972 | Portugal | - | Ireland | 2:1 | ||||
| #57 | 29/06/1972 | Portugal | - | Argentina | 3:1 | |
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| #58 | 02/07/1972 | Portugal | - | Uruguay | 1:1 | ||||
| #59 | 06/07/1972 | Portugal | - | USSR | 1:0 | ||||
| #60 | 09/07/1972 | Brazil | - | Portugal | 1:0 | ||||
| #61 | 02/03/1973 | France | - | Portugal | 1:2 | |
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| #62 | 28/03/1973 | Northern Ireland | - | Portugal | 1:1 | |
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| #63 | 02/05/1973 | Bulgaria | - | Portugal | 2:1 | ||||
| #64 | 13/10/1973 | Portugal | - | Bulgaria | 2:2 |
Mozambique