| #1 | 07/05/1958 | England | - | Portugal | 2:1 | ||||
| #2 | 16/05/1959 | Switzerland | - | Portugal | 4:3 | ||||
| #3 | 11/11/1959 | France | - | Portugal | 5:3 | ||||
| #4 | 27/04/1960 | Germany | - | Portugal | 2:1 | ||||
| #5 | 19/03/1961 | Portugal | - | Luxembourg | 6:0 | ||||
| #6 | 21/05/1961 | Portugal | - | England | 1:1 | ||||
| #7 | 04/06/1961 | Portugal | - | Argentina | 0:2 | ||||
| #8 | 06/05/1962 | Brazil | - | Portugal | 2:1 | ||||
| #9 | 09/05/1962 | Brazil | - | Portugal | 1:0 | ||||
| #10 | 17/05/1962 | Portugal | - | Belgium | 1:2 | ||||
| #11 | 16/12/1962 | Portugal | - | Bulgaria | 3:1 | ||||
| #12 | 21/04/1963 | Portugal | - | Brazil | 1:0 |  |
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| #13 | 29/04/1964 | Switzerland | - | Portugal | 2:3 | |
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| #14 | 03/05/1964 | Belgium | - | Portugal | 1:2 | |
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| #15 | 17/05/1964 | Portugal | - | England | 3:4 | ||||
| #16 | 04/06/1964 | Portugal | - | England | 1:1 | ||||
| #17 | 07/06/1964 | Brazil | - | Portugal | 4:1 | ||||
| #18 | 15/11/1964 | Portugal | - | Spain | 2:1 | ||||
| #19 | 24/01/1965 | Portugal | - | Turkey | 5:1 | ||||
| #20 | 19/04/1965 | Turkey | - | Portugal | 0:1 | ||||
| #21 | 25/04/1965 | CSSR | - | Portugal | 0:1 | ||||
| #22 | 13/06/1965 | Portugal | - | Romania | 2:1 | ||||
| #23 | 24/06/1965 | Portugal | - | Brazil | 0:0 | ||||
| #24 | 31/10/1965 | Portugal | - | CSSR | 0:0 | ||||
| #25 | 21/11/1965 | Romania | - | Portugal | 2:0 | ||||
| #26 | 12/06/1966 | Portugal | - | Norway | 4:0 | |
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| #27 | 18/06/1966 | Scotland | - | Portugal | 0:1 | ||||
| #28 | 26/06/1966 | Portugal | - | Uruguay | 3:0 | ||||
| #29 | 03/07/1966 | Portugal | - | Romania | 1:0 | ||||
| #30 | 13/07/1966 | Portugal | - | Hungary | 3:1 | |
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| #31 | 16/07/1966 | Portugal | - | Bulgaria | 3:0 | ||||
| #32 | 19/07/1966 | Portugal | - | Brazil | 3:1 | ||||
| #33 | 23/07/1966 | Portugal | - | North Korea | 5:3 | |
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| #34 | 26/07/1966 | England | - | Portugal | 2:1 | ||||
| #35 | 28/07/1966 | Portugal | - | USSR | 2:1 | ||||
| #36 | 13/11/1966 | Portugal | - | Sweden | 1:2 | ||||
| #37 | 27/03/1967 | Italy | - | Portugal | 1:1 | ||||
| #38 | 01/06/1967 | Sweden | - | Portugal | 1:1 | ||||
| #39 | 08/06/1967 | Norway | - | Portugal | 1:2 | ||||
| #40 | 12/11/1967 | Portugal | - | Norway | 2:1 | ||||
| #41 | 26/11/1967 | Bulgaria | - | Portugal | 1:0 | ||||
| #42 | 17/12/1967 | Portugal | - | Bulgaria | 0:0 | ||||
| #43 | 30/06/1968 | Portugal | - | Brazil | 0:2 | ||||
| #44 | 27/10/1968 | Portugal | - | Romania | 3:0 | ||||
| #45 | 11/12/1968 | Greece | - | Portugal | 4:2 | |
Portugal